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61.
Jia Dai Xiang Cheng Xiaofeng Li Zhisheng Wang Yufeng Wang Jing Zheng Jun Liu Jiawei Chen Changjin Wu Jinyao Tang 《Advanced functional materials》2021,31(48):2106204
Synthetic active matters are perfect model systems for non-equilibrium thermodynamics and of great potential for novel biomedical and environmental applications. However, most applications are limited by the complicated and low-yield preparation, while a scalable synthesis for highly functional microswimmers is highly desired. In this paper, an all-solution synthesis method is developed where the gold-loaded titania-silica nanotree can be produced as a multi-functional self-propulsion microswimmer. By applying light, heat, and electric field, the Janus nanotree demonstrated multi-mode self-propulsion, including photochemical self-electrophoresis by UV and visible light radiation, thermophoresis by near-infrared light radiation, and induced-charge electrophoresis under AC electric field. Due to the scalable synthesis, the Janus nanotree is further demonstrated as a high-efficiency, low-cost, active adsorbent for water decontamination, where the toxic mercury ions can be reclaimed with enhanced efficiency. 相似文献
62.
Yanqing Zhao Yingli Su Wangcai Zou Gang Chen Yiqing Deng Jun Cheng Haisheng Ren Qiang Zhao 《应用聚合物科学杂志》2021,138(38):50971
In order to prepare waterborne polyurethane with excellent water resistance and thermodynamic properties, a series of side chain fluorinated waterborne polyurethane-urea (FWPU-UA) was synthesized with polytetramethylene ether glycol, N-(2-methyl-1,3-propanediol-2′-)-perfluoro-1-butanesulfonyl amine (NPBA), isophorone diisocyanate, and isophoronediamine. With the increase of NPBA content, the weight loss temperature, glass transition temperature, and tensile strength of FWPU-UA were all improved. Gaussian fitting analysis of infrared data and density functional theory simulation proved that the introduction of fluorine side chains increased the interaction of hydrogen bonding in the FWPU-UA. X-ray photoelectron spectroscopy analysis indicated that the aggregation of fluorine atoms on the surface of film were caused by the migration and enrichment of fluorine side chains. Furthermore, the water resistance of polyurethane-urea film could be significantly improved by adding a small amount of NPBA, and the seven-day water absorption rate of polyurethane-urea film was reduced from 30.13% to 12.55%. 相似文献
63.
Prof. Dr. Chun-Chi Chen Prof. Dr. Jian Min Dr. Lilan Zhang Dr. Yu Yang Prof. Dr. Xuejing Yu Prof. Dr. Rey-Ting Guo 《Chembiochem : a European journal of chemical biology》2021,22(8):1317-1328
Cytochrome P450s are heme-thiolate enzymes that participate in carbon source assimilation, natural compound biosynthesis and xenobiotic metabolism in all kingdoms of life. P450s can catalyze various reactions by using a wide range of organic compounds, thus exhibiting great potential in biotechnological applications. The catalytic reactions of P450s are driven by electron equivalents that are sourced from pyridine nucleotides and delivered by cognate or matching redox partners (RPs). The electron transfer (ET) route from RPs to P450s involves one or more redox center-containing domains. As the rate of ET is one of the main determinants of P450 efficacy, an in-depth understanding of the P450 ET pathway should increase our knowledge of these important enzymes and benefit their further applications. Here, the various P450 RP systems along with current understanding of their ET routes will be reviewed. Notably, state-of-the-art structural studies of the two main types of self-sufficient P450 will also be summarized. 相似文献
64.
Svetlana A. Murzina Polina Yu. Dgebuadze Svetlana N. Pekkoeva Viktor P. Voronin Elena S. Mekhova Nguyen T. H. Thanh 《European Journal of Lipid Science and Technology》2021,123(7):2000321
The sea urchin Diadema setosum is edible and desirable as food by locals in central Vietnam and a promising target for potential fishing. The lipid profiles of the gonads of the sea urchin inhabiting the coastal area in Nha Trang Bay are studied for the first time. The determination of the content of the total lipids (TL), total phospholipids (PL), monoacylglycerols (MAG), diacylglycerols (DAG), triacylglycerols (TAG), cholesterol (Chol), sterol esters, and free fatty acids (FFA) is analyzed by high-performance thin layer chromatography (HPTLC); the phosphatidylserine (PS), phosphatidylethanolamine (PE), phosphatidylinositol (PI), phosphatidylcholine (PC), lysophosphatidylcholine (LPC), and sphingomyelin (SM) are determined by high-pressure liquid chromatography (HPLC); and the fatty acid levels of TLs are identified using gas chromatography (GC). Non-polar TAG, FFA, Chol, and DAG dominated. The content of total PL is significant. PC is abundant among PL fractions, followed by PE, PI, and PS. The TLs contain a high proportion of PUFA, mainly due to arachidonic fatty acid and eicosapentanoic fatty acid. The (n−6)/(n−3) ratio is 1.68, and the atherogenic and thrombogenic indexes of D. setosum are 1.13 and 0.73. The results can be used in the development of marine bioprospecting and methodological approaches for the creation of functional substances. 相似文献
65.
Kuznetsov Yu. A. Markov M. A. Kravchenko I. N. Krasikov A. V. Bykova A. D. 《Refractories and Industrial Ceramics》2021,62(4):421-425
Refractories and Industrial Ceramics - The paper introduces a promising technology for utilizing a traditional scheme for implementing a flow-through micro-arc oxidation method to restore localized... 相似文献
66.
文化、精神以及思想等抽象内涵是紫砂壶艺术魅力的重要组成部分,这是由紫砂壶高雅超逸的艺术特征所决定的,是促进紫砂壶发展的内在动力。“汲浪壶”小巧雅致的身躯中包含着乘风破浪的勇敢无畏,是中华民族精神的一部分,由外在的艺术美过渡至内在的精神表达,体现出民族艺术品格。 相似文献
67.
多堆厂址一级概率安全评价(PSA)研究中,机组数目的增加使得建模工作量剧增,给整个核电厂的风险评估带来困难。结合已有基础,本文研究了多堆厂址始发事件分析的筛选方法,提出利用堆芯损伤频率(CDF)上下限值评估方法,分析厂址内不同机组数对厂址CDF的影响。结果表明,双机组厂址适合优先进行具体分析。针对双机组核电站,对多堆厂址内各始发事件进行筛选。结果表明,丧失厂外电、丧失热阱等事件适合建模分析,并对其他筛选结果给出后续分析建议,为多堆厂址一级PSA后续事故序列建模工作提供了重要基础。 相似文献
68.
69.
Red’kina G. V. Sergienko A. S. Kuznetsov Yu. I. 《Protection of Metals and Physical Chemistry of Surfaces》2021,57(7):1352-1360
Protection of Metals and Physical Chemistry of Surfaces - Abstract—The ability of improving the protective properties of layers formed on zinc in the presence of sodium dodecylphosphonate... 相似文献
70.